I think the earth's atmosphere can have a magnifying effect at low elevations (i.e. when moon is just rising or setting), which makes it appear bigger.
However, depending on what is just below the slice of atmosphere between the observation point and where the light enters the atmosphere can have a significant effect on image quality achievable.
If you're looking across a city, you'll have light, smog and heat pollution to cope with, so it'll be low contrast and wobbling
If you're looking across hot land or a warm sea mass, there could well be thermal disruption alone.
So I guess somewhere out in the middle of nowhere and that is cold, is best, but not Iceland at the moment